How do you Unsync outlook?

outlook.com – remove sync accounts

Under Your app settings, select Mail. In the navigation pane, choose Mail, and under Accounts, select Connected accounts. Select Yes to confirm that you want to stop connecting to the account. After you remove the account from Outlook on the web, you can delete any email messages that still appear in Outlook.

Email in Outlook not syncing in Windows 10; Repair Outlook account

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